Publications

2016
Mikhail A. Kats and Federico Capasso. 2016. “Optical absorbers based on strong interference in ultra-thin films.” LASER & PHOTONICS REVIEWS, 10, 5, Pp. 735-749.Abstract
Optical absorbers find uses in a wide array of applications across the electromagnetic spectrum, including photovoltaic and photochemical cells, photodetectors, optical filters, stealth technology, and thermal light sources. Recent efforts have sought to reduce the footprint of optical absorbers, conventionally based on graded structures or Fabry-Perot-type cavities, by using emerging concepts in plasmonics, metamaterials, and metasurfaces. Unfortunately, these new absorber designs require patterning on subwavelength length scales, and are therefore impractical for many large-scale optical and optoelectronic devices. In this article, we summarize recent progress in the development of optical absorbers based on lossy films with thicknesses significantly smaller than the incident optical wavelength. These structures have a small footprint and require no nanoscale patterning. We outline the theoretical foundation of these absorbers based on ``ultra-thin-film interference'', including the concepts of loss-induced phase shifts and critical coupling, and then review several applications, including ultra-thin color coatings, decorative photovoltaics, high-efficiency photochemical cells, and infrared scene generators.
2016_kats_et_al.pdf
Alan She and Federico Capasso. 2016. “Parallel Polarization State Generation.” SCIENTIFIC REPORTS, 6.Abstract
The control of polarization, an essential property of light, is of wide scientific and technological interest. The general problem of generating arbitrary time-varying states of polarization (SOP) has always been mathematically formulated by a series of linear transformations, i.e. a product of matrices, imposing a serial architecture. Here we show a parallel architecture described by a sum of matrices. The theory is experimentally demonstrated by modulating spatially-separated polarization components of a laser using a digital micromirror device that are subsequently beam combined. This method greatly expands the parameter space for engineering devices that control polarization. Consequently, performance characteristics, such as speed, stability, and spectral range, are entirely dictated by the technologies of optical intensity modulation, including absorption, reflection, emission, and scattering. This opens up important prospects for polarization state generation (PSG) with unique performance characteristics with applications in spectroscopic ellipsometry, spectropolarimetry, communications, imaging, and security.
2016_she_et_al.pdf
M. Khorasaninejad, A. Y. Zhuit, C. Roques-Carmes, W. T. Chen, J. Oh, I. Mishra, R. C. Devlin, and F. Capasso. 2016. “Polarization-Insensitive Metalenses at Visible Wavelengths.” NANO LETTERS, 16, 11, Pp. 7229-7234.Abstract
In this Letter, we demonstrate highly efficient, polarization-insensitive planar lenses (metalenses) at red, green, and blue wavelengths (lambda = 660, 532, and 405 nm). Metalenses with numerical apertures (NA) of 0.85 and 0.6 and corresponding efficiencies as high as 60% and 90% are achieved. These metalenses are less than 600 nm-thick and can focus incident light down to diffraction-limited spots as small as similar to 0.64 lambda and provide high-resolution imaging. In addition, the focal spots are very symmetric with high Strehl ratios. The single step lithography and compatibility with large-scale fabrication processes make metalenses highly promising for widespread applications in imaging and spectroscopy.
2016_khorasaninejad_et_al_1.pdf
D. F. Siriani, C. A. Wang, J. P. Donnelly, M. K. Connors, L. J. Missaggia, D. R. Calawa, D. McNulty, M. C. Zheng, T. S. Mansuripur, and F. Capasso. 2016. “Sensitivity of quantum cascade laser performance to thickness and doping variations.” JOURNAL OF CRYSTAL GROWTH, 452, Pp. 263-267.Abstract
We report on a study of the effects of intentional thickness and doping variations on QCL performance. The measured QCL data had very similar trends to those predicted by an in-house QCL model. It was found that absolute changes to the QCL period had a very small effect on emission wavelength (wave-length/period change < 10 nm/angstrom), whereas the complementary thickness changes between the wells and barriers had a large effect (wavelength/thickness change=550 nm/angstrom). The threshold voltage also changed with these variations and generally agreed well with the model. We show through modeling and experiments that intentional structure variations can have largely different magnitudes of effect on QCL performance. (C) 2015 Elsevier B.V. All rights reserved.
2016_siriani_et_al.pdf
Tobias S. Mansuripur, Camille Vernet, Paul Chevalier, Guillaume Aoust, Benedikt Schwarz, Feng Xie, Catherine Caneau, Kevin Lascola, Chung-en Zah, David P. Caffey, Timothy Day, Leo J. Missaggia, Michael K. Connors, Christine A. Wang, Alexey Belyanin, and Federico Capasso. 2016. “Single-mode instability in standing-wave lasers: The quantum cascade laser as a self-pumped parametric oscillator.” PHYSICAL REVIEW A, 94, 6.Abstract
We report the observation of a clear single-mode instability threshold in continuous-wave Fabry-Perot quantum cascade lasers (QCLs). The instability is characterized by the appearance of sidebands separated by tens of free spectral ranges (FSR) from the first lasing mode, at a pump current not much higher than the lasing threshold. As the current is increased, higher-order sidebands appear that preserve the initial spacing, and the spectra are suggestive of harmonically phase-locked waveforms. We present a theory of the instability that applies to all homogeneously broadened standing-wave lasers. The low instability threshold and the large sideband spacing can be explained by the combination of an unclamped, incoherent Lorentzian gain due to the population grating, and a coherent parametric gain caused by temporal population pulsations that changes the spectral gain line shape. The parametric term suppresses the gain of sidebands whose separation is much smaller than the reciprocal gain recovery time, while enhancing the gain of more distant sidebands. The large gain recovery frequency of the QCL compared to the FSR is essential to observe this parametric effect, which is responsible for the multiple-FSR sideband separation. We predict that by tuning the strength of the incoherent gain contribution, for example by engineering the modal overlap factors and the carrier diffusion, both amplitude-modulated (AM) or frequency-modulated emission can be achieved from QCLs. We provide initial evidence of an AM waveform emitted by a QCL with highly asymmetric facet reflectivities, thereby opening a promising route to ultrashort pulse generation in the mid-infrared. Together, the experiments and theory clarify a deep connection between parametric oscillation in optically pumped microresonators and the single-mode instability of lasers, tying together literature from the last 60 years.
2016_mansuripur_et_al.pdf
Lulu Liu, Simon Kheifets, Vincent Ginis, and Federico Capasso. 2016. “Subfemtonewton Force Spectroscopy at the Thermal Limit in Liquids.” PHYSICAL REVIEW LETTERS, 116, 22.Abstract
We demonstrate thermally limited force spectroscopy using a probe formed by a dielectric microsphere optically trapped in water near a dielectric surface. We achieve force resolution below 1 fN in 100 s, corresponding to a 2 angstrom rms displacement of the probe. Our measurement combines a calibrated evanescent wave particle tracking technique and a lock-in detection method. We demonstrate the accuracy of our method by measurement of the height-dependent force exerted on the probe by an evanescent wave, the results of which are in agreement with Mie theory calculations.
2016_liu_et_al.pdf
M. Khorasaninejad, W. T. Chen, J. Oh, and F. Capasso. 2016. “Super-Dispersive Off-Axis Meta-Lenses for Compact High Resolution Spectroscopy.” NANO LETTERS, 16, 6, Pp. 3732-3737.Abstract
Metasurfaces have opened a new frontier in the miniaturization of optical technology by allowing exceptional control over the wavefront. Here, we demonstrate off-axis meta-lenses that simultaneously focus and disperse light of different wavelengths with unprecedented spectral resolution. They are designed based on the geometric phase via rotated silicon nanofins and can focus light at angles as large as 80. Due to the large angle focusing, these meta-lenses have superdispersive characteristics (0.27 nin/mrad) that make them capable of resolving wavelength differences as small as 200 pm in the telecom region. In addition; by stitching several meta-lenses together, we maintain a high spectral resolution for a wider wavelength range. The meta-lenses have measured efficiencies as high as 90% in the wavelength range of 1.1 to 1.6 mu m. The planar and compact configuration together with high spectral resolution of these meta-lenses has significant potential for emerging portable/wearable optics technology.
2016_khorasaninejad_et_al.pdf
J. P. BALTHASAR MUELLER, KRISTJAN LEOSSON, and Federico Capasso. 2016. “Ultracompact metasurface in-line polarimeter.” OPTICA, 3, 1, Pp. 42-47.Abstract
In-line polarimeters perform nondestructive polarization measurements of optical signals, and play a critical role in monitoring and controlling the polarization environment in, for example, optical networks. While current in-line polarimeters are constructed with multiple optical components, either fabricated into an optical fiber or using free-space optics, we present here a novel architecture conducive to monolithic on-chip integration. This enables the scalable fabrication of high-performance polarization sensors with exceptional stability, compactness, and speed. The method relies on the detection of the highly polarization-dependent scattered field of a subwavelength antenna array known as a metasurface, and is shown here to provide polarization state measurements matching those of a state-of-the-art commercial polarimeter. (C) 2016 Optical Society of America
2016_balthasar_et_al.pdf
2015
Mohammadreza Khorasaninejad, Francesco Aieta, Pritpal Kanhaiya, Mikhail A. Kats, Patrice Genevet, David Rousso, and Federico Capasso. 2015. “Achromatic Metasurface Lens at Telecommunication Wavelengths.” NANO LETTERS, 15, 8, Pp. 5358-5362. Publisher's VersionAbstract
Nanoscale optical resonators enable a new class of flat optical components called metasurfaces. This approach has been used to demonstrate functionalities such as focusing free of monochromatic aberrations (i.e., spherical and coma), anomalous reflection, and large circular dichroism. Recently, dielectric metasurfaces that compensate the phase dispersion responsible for chromatic aberrations have been demonstrated. Here, we utilize an aperiodic array of coupled dielectric nanoresonators to demonstrate a multiwavelength achromatic lens. The focal length remains unchanged for three wavelengths in the near-infrared region (1300, 1550, and 1800 nm). Experimental results are in agreement with full-wave simulations. Our findings are an essential step toward a realization of broadband flat optical elements.
acs_nanolett_5b01727.pdf
Mohammadreza Khorasaninejad and Federico Capasso. 2015. “Broadband Multifunctional Efficient Meta-Gratings Based on Dielectric Waveguide Phase Shifters.” NANO LETTERS, 15, 10, Pp. 6709-6715. Publisher's VersionAbstract
Molding the wavefront of light is a basic principle of any optical design. In conventional optical components such as lenses and waveplates, the wavefront is controlled via propagation phases in a medium much thicker than the wavelength. Metasurfaces instead typically produce the required phase changes using subwavelength-sized resonators as phase shift elements patterned across a surface. This ``flat optics'' approach promises miniaturization and improved performance. Here we introduce metasurfaces which use dielectric ridge waveguides (DRWs) as phase shift elements in which the required phase accumulation is achieved via propagation over a subwavelength distance. By engineering the dispersive response of DRWs, we experimentally realize high resolving power meta-gratings with broadband (lambda = 1.2-1.7 mu m) and efficient routing (splitting and bending) into a single diffraction order, thus overcoming the limits of blazed gratings. In addition, we demonstrate polarization beam splitting capabilities with large suppression ratios.
acs.nanolett.5b02524.pdf
Alejandro W. Rodriguez, Pui-Chuen Hui, David P. Woolf, Steven G. Johnson, Marko Loncar, and Federico Capasso. 2015. “Classical and fluctuation-induced electromagnetic interactions in micron-scale systems: designer bonding, antibonding, and Casimir forces.” ANNALEN DER PHYSIK, 527, 1-2, SI, Pp. 45-80. Publisher's VersionAbstract
Whether intentionally introduced to exert control over particles and macroscopic objects, such as for trapping or cooling, or whether arising from the quantum and thermal fluctuations of charges in otherwise neutral bodies, leading to unwanted stiction between nearby mechanical parts, electromagnetic interactions play a fundamental role in many naturally occurring processes and technologies. In this review, we survey recent progress in the understanding and experimental observation of optomechanical and quantum-fluctuation forces. Although both of these effects arise from exchange of electromagnetic momentum, their dramatically different origins, involving either real or virtual photons, lead to different physical manifestations and design principles. Specifically, we describe recent predictions and measurements of attractive and repulsive optomechanical forces, based on the bonding and antibonding interactions of evanescent waves, as well as predictions of modified and even repulsive Casimir forces between nanostructured bodies. Finally, we discuss the potential impact and interplay of these forces in emerging experimental regimes of micromechanical devices.
johnson_classical_and_fluctuation.pdf
Patrice Genevet, Daniel Wintz, Antonio Ambrosio, Alan She, Romain Blanchard, and Federico Capasso. 2015. “Controlled steering of Cherenkov surface plasmon wakes with a one-dimensional metamaterial.” NATURE NANOTECHNOLOGY, 10, 9, Pp. 804-809. Publisher's VersionAbstract
In the Cherenkov effect a charged particle moving with a velocity faster than the phase velocity of light in the medium radiates light that forms a cone with a half angle determined by the ratio of the two speeds. Here, we show that by creating a running wave of polarization along a one-dimensional metallic nanostructure consisting of subwavelength-spaced rotated apertures that propagates faster than the surface plasmon polariton phase velocity, we can generate surface plasmon wakes, a two-dimensional analogue of Cherenkov radiation. The running wave of polarization travels with a speed determined by the angle of incidence and the photon spin angular momentum of the incident radiation. By changing either one of these properties we demonstrate controlled steering of the Cherenkov surface plasmon wakes.
nnano.2015.137.pdf
Stefan Kalchmair, Romain Blanchard, Tobias S. Mansuripur, Guy-Mael de Naurois, Christian Pfluegl, Mark F. Witinski, Laurent Diehl, Federico Capasso, and Marko Loncar. 2015. “High tuning stability of sampled grating quantum cascade lasers.” OPTICS EXPRESS, 23, 12, Pp. 15734-15747. Publisher's VersionAbstract
Predictable tuning behavior and stable laser operation are both crucial for laser spectroscopy measurements. We report a sampled grating quantum cascade laser (QCL) with high spectral tuning stability over the entire tuning range. We have determined the minimum loss margin required to suppress undesired lasing modes in order to ensure predictable tuning behavior. We have quantified power fluctuations and drift of our devices by measuring the Allan deviation. To demonstrate the feasibility of sampled grating QCLs for high-precision molecular spectroscopy, we have built a simple transmission spectroscopy setup. Our results prove that sampled grating QCLs are suitable light sources for highly sensitive spectroscopy measurements. (C) 2015 Optical Society of America
oe-23-12-15734.pdf
Daniel Wintz, Patrice Genevet, Antonio Ambrosio, Alex Woolf, and Federico Capasso. 2015. “Holographic Metalens for Switchable Focusing of Surface Plasmons.” NANO LETTERS, 15, 5, Pp. 3585-3589. Publisher's VersionAbstract
Surface plasmons polaritons (SPPs) are light like waves confined to the interface between a metal and a dielectric. Excitation and control of these modes requires components such as couplers and lenses. We present the design of a new lens based on holographic principles. The key feature is the ability to switchably control SPP focusing by changing either the incident wavelength or polarization. Using phase-sensitive near-field imaging of the surface plasmon wavefronts, we have observed their switchable focusing and steering as the wavelength or polarization is changed.
acs.nanolett.5b01076.pdf
Patrice Genevet and Federico Capasso. 2015. “Holographic optical metasurfaces: a review of current progress.” REPORTS ON PROGRESS IN PHYSICS, 78, 2.Abstract
In this article, we review recent developments in the field of surface electromagnetic wave holography. The holography principle is used as a tool to solve an inverse engineering problem consisting of designing novel plasmonic interfaces to excite either surface waves or free-space beams with any desirable field distributions. Leveraging on the new nanotechnologies to carve subwavelength features within the large diffracting apertures of conventional holograms, it is now possible to create binary holographic interfaces to shape both amplitude phase and polarization of light. The ability of the new generation of ultrathin and compact holographic optical devices to fully address light properties could find widespread applications in photonics.
genevet_2015_rep._prog._phys._78_024401.pdf
Tobias S. Mansuripur, Guy-Mael de Naurois, Alexey Belyanin, and Federico Capasso. 2015. “Lasers with distributed loss have a sublinear output power characteristic.” OPTICA, 2, 1, Pp. 48-55. Publisher's VersionAbstract
It is a generally accepted fact of laser physics that in a homogeneously broadened gain medium, above threshold the output power of the laser grows linearly with the pump power. The derivation requires only a few simple lines in laser textbooks, and the linear growth is a direct result of the fact that above threshold, the intracavity optical intensity will increase to the point that the gain is saturated to the level of the net loss-so-called gain pinning or clamping. Such a derivation, however, assumes that the mirror loss is distributed (the approximation of uniform gain saturation) which is only a good assumption for cavities whose end mirrors have reflectivities close to one. Furthermore, in gain media with a distributed loss there is a maximum achievable intracavity intensity that in turn limits the output power. We show that the approximation of uniform gain saturation leads to output powers that violate this limit. More generally, for lasers with low mirror reflectivities that also have distributed loss, we prove that the output power grows sub-linearly with the pump power close to threshold. Furthermore, after threshold the output grows linearly, but with a slope efficiency that can be substantially smaller than predicted by the uniform gain saturation theory, with the largest deviation occurring for traveling-wave lasers and asymmetric Fabry-Perot lasers. These results are particularly applicable to semiconductor lasers, and specific applications to quantum cascade lasers are discussed. (C) 2015 Optical Society of America
optica-2-1-48.pdf
Amaury Hayat, J. P. BALTHASAR MUELLER, and Federico Capasso. 2015. “Lateral chirality-sorting optical forces.” PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 112, 43, Pp. 13190-13194. Publisher's VersionAbstract
The transverse component of the spin angular momentum of evanescent waves gives rise to lateral optical forces on chiral particles, which have the unusual property of acting in a direction in which there is neither a field gradient nor wave propagation. Because their direction and strength depends on the chiral polarizability of the particle, they act as chirality-sorting and may offer a mechanism for passive chirality spectroscopy. The absolute strength of the forces also substantially exceeds that of other recently predicted sideways optical forces.
13190.full_.pdf
Mark F. Witinski, Romain Blanchard, Christian Pfluegl, Laurent Diehl, Biao Li, Benjamin Pancy, Daryoosh Vakhshoori, and Federico Capasso. 2015. “Monolithic DFB QCL array aims at handheld IR spectral analysis.” LASER FOCUS WORLD, 51, 11, Pp. 36-39. Publisher's VersionAbstract
Many QCLs combined on a single chip demonstrate fully electronic wavelength tuning for stand-off IR spectroscopy of explosives and other materials.
laserfocusworldqclarrays.pdf
Francesco Aieta, Mikhail A. Kats, Patrice Genevet, and Federico Capasso. 2015. “Multiwavelength achromatic metasurfaces by dispersive phase compensation.” SCIENCE, 347, 6228, Pp. 1342-1345. Publisher's VersionAbstract
The replacement of bulk refractive optical elements with diffractive planar components enables the miniaturization of optical systems. However, diffractive optics suffers from large chromatic aberrations due to the dispersion of the phase accumulated by light during propagation. We show that this limitation can be overcome with an engineered wavelength-dependent phase shift imparted by a metasurface, and we demonstrate a design that deflects three wavelengths by the same angle. A planar lens without chromatic aberrations at three wavelengths is also presented. Our designs are based on low-loss dielectric resonators, which introduce a dense spectrum of optical modes to enable dispersive phase compensation. The suppression of chromatic aberrations in metasurface-based planar photonics will find applications in lightweight collimators for displays, as well as chromatically corrected imaging systems.
2015_aieta_et_al.pdf
Patrick Rauter and Federico Capasso. 2015. “Multi-wavelength quantum cascade laser arrays.” LASER & PHOTONICS REVIEWS, 9, 5, Pp. 452-477.Abstract
The progress on multi-wavelength quantum cascade laser arrays in the mid-infrared is reviewed, which are a powerful, robust and versatile source for next-generation spectroscopy and stand-off detection systems. Various approaches for the array elements are discussed, from conventional distributed-feedback lasers over master-oscillator power-amplifier devices to tapered oscillators, and the performances of the different array types are compared. The challenges associated with reliably achieving single-mode operation at deterministic wavelengths for each laser element in combination with a uniform distribution of high output power across the array are discussed. An overview of the range of applications benefiting from the quantum cascade laser approach is given. The distinct and crucial advantages of arrays over external cavity quantum cascade lasers as tunable single-mode sources in the mid-infrared are discussed. Spectroscopy and hyperspectral imaging demonstrations by quantum cascade laser arrays are reviewed.
lpor.201500095.pdf

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