Publications

2017
Daniel Wintz, Antonio Ambrosio, Alexander Y. Zhu, Patrice Genevet, and Federico Capasso. 2017. “Anisotropic Surface Plasmon Polariton Generation Using Bimodal V-Antenna Based Metastructures.” ACS PHOTONICS, 4, 1, Pp. 22-27.Abstract
V-shaped nanoantennas are among the popular choices for the unit element of a metasurface, a nanostructured surface used for its ability to mold and control the wavefront of light. In general, the motivation for choosing the V-antenna as the unit element comes from its bimodal nature, where the introduction of the second mode offers extra control over the scattered wavefronts. Here, through near-field scanning optical microscopy, we study a 1D metastructure comprised of V-antennas in the context of generating asymmetric surface plasmon polariton (SPP) wavefronts. The key point is that the use of the V-antenna allows for the creation of a two-dimensional phase gradient with a single line of antennas, where the extra phase dimension offers additional control and allows for asymmetric features. Two different asymmetries are created: (1) SPP wavefronts that have different propagation directions on either side of the metastructure, and (2) SPP wavefront asymmetry through focusing: one side of the metastructure focuses SPP wavefronts, while the other side has diverging SPP wavefronts.
acsphotonics.6b00758.pdf
Robert C. Devlin, Antonio Ambrosio, Noah A. Rubin, Balthasar Mueller, and Federico Capasso. 2017. “Arbitrary spin-to-orbital angular momentum conversion of light.” Science, 358, 6365, Pp. 896-900.Abstract
Optical elements that convert the spin angular momentum (SAM) of light into vortex beams have found applications in classical and quantum optics. These elements-SAM-toorbital angular momentum (OAM) converters-are based on the geometric phase and only permit the conversion of left-and right-circular polarizations (spin states) into states with opposite OAM. We present a method for converting arbitrary SAM states into total angular momentum states characterized by a superposition of independent OAM. We designed a metasurface that converts left-and right-circular polarizations into states with independent values of OAM and designed another device that performs this operation for elliptically polarized states. These results illustrate a general material-mediated connection between SAM and OAM of light and may find applications in producing complex structured light and in optical communication.
science.full_.pdf
Vishal Jain, Magnus Heurlin, Mohammad Karimi, Laiq Hussain, Mahtab Aghaeipour, Ali Nowzari, Alexander Berg, Gustav Nylund, Federico Capasso, Lars Samuelson, Magnus T. Borgstroem, and Hakan Pettersson. 2017. “Bias-dependent spectral tuning in InP nanowire-based photodetectors.” Nanotechnology, 28, 11.Abstract
Nanowire array ensembles contacted in a vertical geometry are extensively studied and considered strong candidates for next generations of industrial scale optoelectronics. Key challenges in this development deal with optimization of the doping profile of the nanowires and the interface between nanowires and transparent top contact. Here we report on photodetection characteristics associated with doping profile variations in InP nanowire array photodetectors. Bias-dependent tuning of the spectral shape of the responsivity is observed which is attributed to a Schottky-like contact at the nanowire-ITO interface. Angular dependent responsivity measurements, compared with simulated absorption spectra, support this conclusion. Furthermore, electrical simulations unravel the role of possible self-gating effects in the nanowires induced by the ITO/SiOx wrap-gate geometry. Finally, we discuss possible reasons for the observed low saturation current at large forward biases.
jain_2017_nanotechnology.pdf
Lulu Liu, Simon Kheifets, Vincent Ginis, Andrea Di Donato, and Federico Capasso. 2017. “Elliptical orbits of microspheres in an evanescent field.” PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 114, 42, Pp. 11087-11091.Abstract
We examine the motion of periodically driven and optically tweezed microspheres in fluid and find a rich variety of dynamic regimes. We demonstrate, in experiment and in theory, that mean particle motion in 2D is rarely parallel to the direction of the applied force and can even exhibit elliptical orbits with non-zero orbital angular momentum. The behavior is unique in that it depends neither on the nature of the microparticles nor that of the excitation; rather, angular momentum is introduced by the particle's interaction with the anisotropic fluid and optical trap environment. Overall, we find this motion to be highly tunable and predictable.
1714953114.full_.pdf
Jura Rensberg, You Zhou, Steffen Richter, Chenghao Wan, Shuyan Zhang, Philipp Schoppe, Rdiger Schmidt-Grund, Shriram Ramanathan, Federico Capasso, Mikhail A. Kats, and Carsten Ronning. 2017. “Epsilon-Near-Zero Substrate Engineering for Ultrathin-Film Perfect Absorbers.” PHYSICAL REVIEW APPLIED, 8, 1.Abstract
Efficient suppression of reflection is a key requirement for perfect absorption of light. Recently, it has been shown that reflection can be effectively suppressed utilizing a single ultrathin film deposited on metals or polar materials featuring phonon resonances. The wavelength at which reflection can be fully suppressed is primarily determined by the nature of these substrates and is pinned to particular values near plasma or phonon resonances-the former typically in the ultraviolet or visible and the latter in the infrared. Here, we explicitly identify the required optical properties of films and substrates for the design of absorbing antireflection coatings based on ultrathin films. We find that completely suppressed reflection using films with thicknesses much smaller than the wavelength of light occurs within a spectral region where the real part of the refractive index of the substrate is n less than or similar to 1, which is characteristic of materials with permittivity close to zero. We experimentally verify this condition by using an ultrathin vanadium dioxide film with dynamically tunable optical properties on several epsilon-near-zero materials, including aluminum-doped zinc oxide. By tailoring the plasma frequency of the aluminum-doped zinc oxide, we are able to tune the epsilon-near-zero point, thus achieving suppressed reflection and near-perfect absorption at wavelengths that continuously span the near-infrared and long-wave midinfrared ranges.
physrevapplied.8.014009.pdf
Wei Ting Chen, Mohammadreza Khorasaninejad, Alexander Y. Zhu, Jaewon Oh, Robert C. Devlin, Aun Zaidi, and Federico Capasso. 2017. “Generation of wavelength-independent subwavelength Bessel beams using metasurfaces.” Light Science and Applications, 6.Abstract
Bessel beams are of great interest due to their unique non-diffractive properties. Using a conical prism or an objective paired with an annular aperture are two typical approaches for generating zeroth-order Bessel beams. However, the former approach has a limited numerical aperture (NA), and the latter suffers from low efficiency, as most of the incident light is blocked by the aperture. Furthermore, an additional phase-modulating element is needed to generate higher-order Bessel beams, which in turn adds complexity and bulkiness to the system. We overcome these problems using dielectric metasurfaces to realize meta-axicons with additional functionalities not achievable with conventional means. We demonstrate meta-axicons with high NA up to 0.9 capable of generating Bessel beams with full width at half maximum about as small as similar to lambda/3 (lambda = 405 nm). Importantly, these Bessel beams have transverse intensity profiles independent of wavelength across the visible spectrum. These meta-axicons can enable advanced research and applications related to Bessel beams, such as laser fabrication, imaging and optical manipulation.
lsa2016259.pdf
J. William Boley, Kundan Chaudhary, Thomas J. Ober, Mohammadreza Khorasaninejad, Wei Ting Chen, Erik Hanson, Ashish Kulkarni, Jaewon Oh, Jinwoo Kim, Larry K. Aagesen, Alexander Y. Zhu, Federico Capasso, Katsuyo Thornton, Paul V. Braun, and Jennifer A. Lewis. 2017. “High-Operating-Temperature Direct Ink Writing of Mesoscale Eutectic Architectures.” ADVANCED MATERIALS, 29, 7, Pp. 1604778.Abstract
High-operating-temperature direct ink writing (HOT-DIW) of mesoscale architectures that are composed of eutectic silver chloride-potassium chloride. The molten ink undergoes directional solidification upon printing on a cold substrate. The lamellar spacing of the printed features can be varied between approximately 100 nm and 2 mu m, enabling the manipulation of light in the visible and infrared range.
adma.201604778.pdf
Wei Ting Chen, Alexander Y. Zhu, Mohammadreza Khorasaninejad, Zhujun Shi, Vyshakh Sanjeev, and Federico Capasso. 2017. “Immersion Meta-Lenses at Visible Wavelengths for Nanoscale Imaging.” Nano Letters, 17, 5, Pp. 3188-3194.Abstract
Immersion objectives can focus light into a spot smaller than what is achievable in free space, thereby enhancing the spatial resolution for various applications such as microscopy, spectroscopy, and lithography. Despite the availability of advanced lens polishing techniques, hand-polishing is still required to manufacture the front lens of a high-end immersion objective, which poses major constraints for lens design. This limits the shape of the front lens to spherical. Therefore, several other lenses need to be cascaded to correct for spherical aberration, resulting in significant challenges for miniaturization and adding design complexity for different immersion liquids. Here, by using metasurfaces, we demonstrate liquid immersion meta-lenses free of spherical aberration at various design wavelengths in the visible spectrum. We report water and oil immersion meta-lenses of various numerical apertures (NA) up to 1.1 and show that their measured focal spot sizes are diffraction-limited with Strehl ratios of approximately 0.9 at 532 nm. By integrating the oil immersion meta-lens (NA = 1.1) into a commercial scanning confocal microscope, we achieve an imaging spatial resolution of approximately 200 nm. These meta-lenses can be easily adapted to focus light through multilayers of different refractive indices and mass-produced using modern industrial manufacturing or nanoimprint techniques, leading to cost-effective high-end optics.
acs.nanolett.7b00717.pdf
Vishal Jain, Magnus Heurlin, Enrique Barrigon, Lorenzo Bosco, Ali Nowzari, Shishir Shroff, Virginia Boix, Mohammad Karimi, Reza J. Jam, Alexander Berg, Lars Samuelson, Magnus T. Borgstrom, Federico Capasso, and Hakan Pettersson. 2017. “InP/InAsP Nanowire-Based Spatially Separate Absorption and Multiplication Avalanche Photodetectors.” ACS Photonics , 4, 11, Pp. 2693-2698.Abstract
Avalanche photodetectors (APDs) are key components in optical communication systems due to their increased photocurrent gain and short response time as compared to conventional photo-detectors. A detector design where the multiplication region is implemented in a large band gap material is desired to avoid detrimental Zener tunneling leakage currents, a concern otherwise in smaller band gap materials required for absorption at 1.3/1.55 mu m. Self-assembled III-V semiconductor nanowires offer key advantages such as enhanced absorption due to optical resonance effects, strain-relaxed hetero-2 structures, and compatibility with mainstream silicon technology. Here, we present electrical and optical characteristics of single InP and InP/InAsP nanowire APD structures. Temperature-dependent breakdown characteristics of p(+)-n-n(+) InP nanowire devices were investigated first. A clear trap-induced shift in breakdown voltage was inferred from I-V measurements. An improved contact formation to the p(+)-InP segment was observed upon annealing, and its effect on breakdown characteristics was investigated. The band gap in the absorption region was subsequently varied from pure InP to InAsP to realize spatially separate absorption and multiplication APDs in heterostructure nanowires. In contrast to the homojunction APDs, no trap-induced shifts were observed for the heterostructure APDs. A gain of 12 was demonstrated for selective optical excitation of the InAsP segment. Additional electron beam-induced current measurements were carried out to investigate the effect of local excitation along the nanowire on the I-V characteristics. Simulated band profiles and electric field distributions support our interpretation of the experiments. Our results provide important insight for optimization of avalanche photodetector devices based on III-V nanowires.
acsphotonics.7b00389.pdf
Federico Capasso, Paul Corkum, Olga Kocharovskaya, Lev Pitaevskii, and Michael V. Sadovskii. 2017. “Leonid Keldysh OBITUARY.” PHYSICS TODAY, 70, 6, Pp. 75-76. pt.3.3605.pdf
Henning Galinski, Andrea Fratalocchi, Max Dobeli, and Federico Capasso. 2017. “Light Manipulation in Metallic Nanowire Networks with Functional Connectivity.” Advanced Optical Materials, 5, 5. adom.201600580.pdf
Antonio Ambrosio, Luis A. Jauregui, Siyuan Dai, Kundan Chaudhary, Michele Tamagnone, Michael M. Fogler, Dimitri N. Basov, Federico Capasso, Philip Kim, and William L. Wilson. 2017. “Mechanical Detection and Imaging of Hyperbolic Phonon Polaritons in Hexagonal Boron Nitride.” ACS NANO, 11, 9, Pp. 8741-8746.Abstract
Mid-infrared nanoimaging and spectroscopy of two-dimensional (2D) materials have been limited so far to scattering-type scanning near-field optical microscopy (s-SNOM) experiments, where light from the sample is scattered by a metallic-coated atomic force microscope (AFM) tip interacting with the material at the nanoscale. These experiments have recently allowed imaging of plasmon polaritons in graphene as well as hyperbolic phonon polaritons in hexagonal boron nitride (hBN). Here we show that the high mechanical sensitivity of an AFM cantilever can be exploited for imaging hyperbolic phonon polaritons in hBN. In our imaging process, the lattice vibrations of hBN micrometer-sized flakes are locally enhanced by the launched phonon polaritons. These enhanced vibrations are coupled to the AFM tip in contact with the sample surface and recorded during scanning. Imaging resolution of Delta/20 is shown (Delta being the polaritonic fringes' separation distance), comparable to the best resolution in s-SNOM. Importantly, this detection mechanism is free from light background, and it is in fact the first photonless detection of phonon polaritons.
2017_ambrosio_et_al_acs_nano.pdf
Benedikt Groever, Wei Ting Chen, and Federico Capasso. 2017. “Meta-Lens Doublet in the Visible Region.” Nano Letters, 17, 8, Pp. 4902-4907.Abstract
Recently, developments in meta-surfaces have allowed for the possibility of a fundamental shift in lens manufacturing from the century-old grinding technology to nanofabrication opening a way toward mass producible high-end meta-lenses. Inspired by early camera lenses and to overcome the aberrations of planar single-layered meta-lenses, we demonstrate a compact meta lens doublet by patterning two metasurfaces on both sides of a substrate. This meta-lens doublet has a numerical aperture of 0.44, a focal length of 342.5 mu m, and a field of view of 50 that enables diffraction-limited monochromatic imaging along the focal plane at a wavelength of 532 mu. The compact design has various imaging applications in microscopy, machine vision, and computer vision.
acs.nanolett.7b01888.pdf
Mohammadreza Khorasaninejad and Federico Capasso. 2017. “Metalenses: Versatile multifunctional photonic components.” Science, 358, 6367.Abstract
Recent progress in metasurface designs fueled by advanced-fabrication techniques has led to the realization of ultrathin, lightweight, and flat lenses (metalenses) with unprecedented functionalities. Owing to straightforward fabrication, generally requiring a single-step lithography, and the possibility of vertical integration, these planar lenses can potentially replace or complement their conventional refractive and diffractive counterparts, leading to further miniaturization of high-performance optical devices and systems. Here we provide a brief overview of the evolution of metalenses, with an emphasis on the visible and near-infrared spectrum, and summarize their important features: diffraction-limited focusing, high-quality imaging, and multifunctionalities. We discuss impending challenges, including aberration correction, and also examine current issues and solutions. We conclude by providing an outlook of this technology platform and identifying promising directions for future research.
eaam8100.full_1.pdf
J. P. BALTHASAR MUELLER, Noah A. Rubin, Robert C. Devlin, Benedikt Groever, and Federico Capasso. 2017. “Metasurface Polarization Optics: Independent Phase Control of Arbitrary Orthogonal States of Polarization.” Physical Review Letters, 118, 11, Pp. 113901.Abstract
We present a method allowing for the imposition of two independent and arbitrary phase profiles on any pair of orthogonal states of polarization-linear, circular, or elliptical-relying only on simple, linearly birefringent wave plate elements arranged into metasurfaces. This stands in contrast to previous designs which could only address orthogonal linear, and to a limited extent, circular polarizations. Using this approach, we demonstrate chiral holograms characterized by fully independent far fields for each circular polarization and elliptical polarization beam splitters, both in the visible. This approach significantly expands the scope of metasurface polarization optics.
physrevlett.118.113901_1.pdf
Christine A. Wang, Benedikt Schwarz, Dominic F. Siriani, Leo J. Missaggia, Michael K. Connors, Tobias S. Mansuripur, Daniel R. Calawa, Daniel McNulty, Michael Nickerson, Joseph P. Donnelly, Kevin Creedon, and Federico Capasso. 2017. “MOVPE Growth of LWIR AlInAs/GaInAs/InP Quantum Cascade Lasers: Impact of Growth and Material Quality on Laser Performance.” IEEE Journal of Selected Topics in Quantum Electronics, 23, 6.Abstract
The quality of epitaxial layers in quantum cascade lasers (QCLs) has a primary impact on QCL performance, and establishing correlations between epitaxial growth and materials properties is of critical importance for continuing improvements. We present an overview of the growth challenges of these complex QCL structures; describe the metalorganic vapor phase epitaxy growth of AlInAs/GaInAs/InP QCL materials; discuss materials properties that impact QCL performance; and investigate various QCL structure modifications and their effects on QCL performance. We demonstrate uncoated buried-heterostructure 9.3-mu m QCLs with 1.32-W continuous-wave output power and maximum wall plug efficiency (WPE) of 6.8%. This WPE is more than 50% greater than previously reportedWPEs for unstrained QCLs emitting at 8.9 mu m and only 30% below strained QCLs emitting around 9.2 mu m.
07870635.pdf
Stefano Luigi Oscurato, Fabio Borbone, Robert Charles Devlin, Federico Capasso, Pasqualino Maddalena, and Antonio Ambrosio. 2017. “New microscopy technique based on position localization of scattering particles.” Optics Express, 25, 10, Pp. 11530-11549.Abstract
We introduce the Holographic - Single Scatterer Localization Microscopy in which we combine dynamical laser speckle illumination with centroid localization of backscattered light spots in order to localize isolated scattering particles. The reconstructed centroid images show very accurate particle localization, with precision much better than the width of diffraction-limited image of the particles recorded by the CCD. Furthermore, the method provides an improved resolution in distinguishing two very close scattering objects compared to the standard laser scanning techniques and can be assimilated to a confocal technique in the ability of light background rejection in three-dimensional disposition of scattering objects. The illumination is controlled via a digital holography setup based on the use of a spatial light modulator. This allows not only a high level of versatility in the illumination patterns, but also the remarkable characteristics of absence of moving mechanical parts, typical of the laser scanning techniques, and the possibility of strongly miniaturizing the setup. (C) 2017 Optical Society of America
oe-25-10-11530.pdf
Antonio Ambrosio, Robert Charles Devlin, Federico Capasso, and William L. Wilson. 2017. “Observation of Nanoscale Refractive Index Contrast via Photoinduced Force Microscopy.” ACS Photonics, 4, 4, Pp. 846-851.Abstract
Near-field optical microscopy (NSOM) is a scanning probe technique that allows optical imaging of sample surfaces with nanoscale resolution. Generally, all NSOM schemes rely on illuminating the sample surface and collecting the localized scattered light resulting from the interaction of the microscopes nanoscale probe with the sample surface in the illuminated region. Currently, a new set of nanospectroscopic techniques are being developed using Atomic Force Microscopes to detect optical interactions without detecting any light. One of these approaches is photoinduced force microscopy (PiFM), where local optical forces, originated by the illumination of the tip sample region, are mechanically detected as forced oscillations of the cantilever of an atomic microscope operating in a multifrequency mode. In this article we show high resolution nanoimaging via PiFM with a contrast only related to the local refractive index of a sample specifically designed to unambiguously decouple morphology from optical response at the nanoscale. Imaging lateral resolution better than 10 nm is obtained, and the optimization of the contrast mechanism is described. Our results represent a step forward in understanding the potential of the PiFM technique, showing the possibility of high resolution imaging of the local polarizability of the sample and subsequently using the mechanism to explore complex spectral behavior at the nanoscale.
acsphotonics.6b00911_1.pdf
Henning Galinski, Andrea Fratalocchi, Max Döbeli, and Federico Capasso. 2017. “Optical Nanomaterials: Light Manipulation in Metallic Nanowire Networks with Functional Connectivity.” Advanced Optical Materials, 5, 5. Publisher's VersionAbstract
In article number 1600580, Andrea Fratalocchi, Federico Capasso, and co-workers introduce a novel class of “network” metamaterials, whose functionality is controlled by the connectivity among heterogeneous subwavelength components within a complex network. Using theory and experiments in dealloyed metallic nanowire networks, it is shown how the network connectivity supports the formation of a tunable absorbing state, which is deterministically controllable and originates in regions that are only a few nanometers thick.
adom.201770027.pdf
Stefan Schoche, Nina Hong, Mohammadreza Khorasaninejad, Antonio Ambrosio, Emanuele Orabona, Pasqualino Maddalena, and Federico Capasso. 2017. “Optical properties of graphene oxide and reduced graphene oxide determined by spectroscopic ellipsometry.” Applied Surface Science, 421, B, SI, Pp. 778-782.Abstract
We report the optical constants of graphene oxide and reduced graphene oxide determined by spectroscopic ellipsometry. The dynamic changes in optical properties and thickness of a drop-cast graphene oxide layer during reduction by long-term exposure to focused broad-band white light are monitored in situ. The anisotropic optical constants of the graphene oxide layer and the isotropically averaged optical constants of the reduced layer are precisely determined from a multiple-location analysis of spatially resolved data across the exposed location and a multiple-time-step analysis of the dynamic data, respectively. Observed inter-band transitions in the graphene oxide layer are discussed in relation to theoretical predictions for different coverage levels of the graphene oxide sheets with oxygen containing functional groups. The derived optical constants of the reduced graphene oxide layer are compared to reported values of graphene and thermally reduced graphene oxide. (C) 2017 Elsevier B.V. All rights reserved.
2017_schoche_et_al.pdf

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